Abstract: We develop a periodically-poled LiNbO3 (PPLN)
device for highly-efficient third-harmonic generation (THG), where
the THG efficiency is enhanced with a cavity. THG can usually be
produced via χ(3)-nonlinear materials by optical pumping with very
high pump-power. Instead, we here propose THG by moderate-power
pumping through a specially-designed PPLN device containing
only χ(2)-nonlinearity, where sum-frequency generation in the χ(2)
process is employed for the mixing of a pump beam and a
second-harmonic-generation (SHG) beam produced from the pump
beam. The cavity is designed to increase the SHG power with dichroic
mirrors attached to both ends of the device that perfectly reflect
the SHG beam back to the device and yet let the pump and THG
beams pass through the mirrors. This brings about a THG-power
enhancement because of THG power proportional to the enhanced
SHG power. We examine the THG-efficiency dependence on the
mirror reflectance and show that very high THG-efficiency is obtained
at moderate pump-power when compared with that of a cavity-free
PPLN device.